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I also find Firefox’s UI/UX to be much better, especially the settings UI. On Firefox it’s easier to find a setting you want by just heading to the category and scrolling down. This way you immediately see all of the setting options and you don’t need to head through a maze of submenus.
With Chrome you don’t have a few broad categories for what you’re looking for. Instead you have many vague categories with lots of submenus.